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TVT, 2010, Volume 48, Issue 4, Pages 531–535 (Mi tvt765)  

Thermophysical Properties of Materials

Development and experimental verification of a method for assessment of consistency of the thermodynamic and structural properties of binary coolants based on systems of alkali metals

D. N. Kagan, G. A. Krechetova, É. Shpil'rain

Joint Institute for High Temperatures, Russian Academy of Sciences, Moscow

Abstract: The construction of correlation function of concentration fluctuations $S_{cc}(0) = f(T, x_i)$ is used to validate the criterion of assessment of the internal consistency of the thermodynamic and structural properties of liquid-metal alloys, as well as of the reliability of experimental data on the Gibbs energy of solution formation $\Delta G$, methods of their approximation, and theoretical models which reproduce the behavior of $\Delta G$. The method is verified for the Cs—Na, K—Na, and Cs—K systems of alkali metals using the data of thermodynamic experiment in determining the Gibbs energy of formation of liquid-metal solution $\Delta G$ which is the basis for construction of the function $S_{cc}(0)$. The data on statistical structure factor $S(0)$ uniquely related to function $S_{cc}(0)$ are obtained using the results (available in the literature) of experiments in X-ray and neutron spectroscopy, including data on diffraction and small-angle inelastic scattering.

Full text: PDF file (478 kB)

English version:
High Temperature, 2010, 48:4, 506–510

Bibliographic databases:

UDC: 536.777+621.039.534+669.017.13
Received: 20.05.2009

Citation: D. N. Kagan, G. A. Krechetova, É. Shpil'rain, “Development and experimental verification of a method for assessment of consistency of the thermodynamic and structural properties of binary coolants based on systems of alkali metals”, TVT, 48:4 (2010), 531–535; High Temperature, 48:4 (2010), 506–510

Citation in format AMSBIB
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\by D.~N.~Kagan, G.~A.~Krechetova, \'E.~Shpil'rain
\paper Development and experimental verification of a method for assessment of consistency of the thermodynamic and structural properties of binary coolants based on systems of alkali metals
\jour TVT
\yr 2010
\vol 48
\issue 4
\pages 531--535
\mathnet{http://mi.mathnet.ru/tvt765}
\transl
\jour High Temperature
\yr 2010
\vol 48
\issue 4
\pages 506--510
\crossref{https://doi.org/10.1134/S0018151X10040073}
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\scopus{http://www.scopus.com/record/display.url?origin=inward&eid=2-s2.0-77955754199}


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