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UFN, 2011, Volume 181, Number 4, Pages 365–387 (Mi ufn2361)  

This article is cited in 16 scientific papers (total in 16 papers)


Kinetic methods for measuring the temperature of clusters and nanoparticles in molecular beams

G. N. Makarov

Institute of Spectroscopy, Russian Academy of Sciences

Abstract: The temperature (internal energy) of clusters and nanoparticles is an important physical parameter which affects many of their properties and the character of processes they are involved in. At the same time, determining the temperature of free clusters and nanoparticles in molecular beams is a rather complicated problem because the temperature of small particles depends on their size. In this paper, recently developed kinetic methods for measuring the temperature of clusters and nanoparticles in molecular beams are reviewed. The definition of temperature in the present context is given, and how the temperature affects the properties of and the processes involving the particles is discussed. The temperature behavior of clusters and nanoparticles near a phase transition point is analyzed. Early methods for measuring the temperature of large clusters are briefly described. It is shown that, compared to other methods, new kinetic methods are more universal and applicable for determining the temperature of clusters and nanoparticles of practically any size and composition. The future development and applications of these methods are outlined.


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English version:
Physics–Uspekhi, 2011, 54:4, 351–370

Bibliographic databases:

PACS: 07.77.Gx, 36.40.-c, 36.40.Ei, 42.62.Fi, 81.07.Nb, 82.50.Hp
Received: April 21, 2010
Revised: June 17, 2010

Citation: G. N. Makarov, “Kinetic methods for measuring the temperature of clusters and nanoparticles in molecular beams”, UFN, 181:4 (2011), 365–387; Phys. Usp., 54:4 (2011), 351–370

Citation in format AMSBIB
\by G.~N.~Makarov
\paper Kinetic methods for measuring the temperature of clusters and nanoparticles in molecular beams
\jour UFN
\yr 2011
\vol 181
\issue 4
\pages 365--387
\jour Phys. Usp.
\yr 2011
\vol 54
\issue 4
\pages 351--370

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    2. Valentin M. Apatin, Valery N. Lokhman, Danil D. Ogurok, Denis G. Poydashev, Evgeny A. Ryabov, “Photodissociation of IF2CCOF clusters by resonant IR radiation”, Eur. Phys. J. D, 67:3 (2013), 66  crossref  isi  scopus
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    7. M. Basire, J.-M. Soudan, C. Angelié, “Nanothermodynamics of large iron clusters by means of a flat histogram Monte Carlo method”, J. Chem. Phys, 141:10 (2014), 104304  crossref  isi  scopus
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    10. D.G.. Poydashev, V.N.. Lokhman, V.O.. Kompanets, S.V.. Chekalin, E.A.. Ryabov, “Ultrafast Dissociation Dynamics of [Fe(CO)5]nClusters Induced by Femtosecond IR Radiation”, J. Phys. Chem. A, 2014, 1411121120  crossref  isi  scopus
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    14. Kompanets V.O. Lokhman V.N. Poydashev D.G. Chekalin S.V. Ryabov E.A., “Dynamics of photoprocesses induced by femtosecond infrared radiation in free molecules and clusters of iron pentacarbonyl”, J. Exp. Theor. Phys., 122:4 (2016), 621–632  crossref  isi  elib  scopus
    15. G. N. Makarov, “Laser IR fragmentation of molecular clusters: the role of channels for energy input and relaxation, the influence of surroundings, and the dynamics of fragmentation”, Phys. Usp., 60:3 (2017), 227–258  mathnet  crossref  crossref  adsnasa  isi  elib
    16. G. N. Makarov, “Control of the parameters and composition of molecular and cluster beams by means of IR lasers”, Phys. Usp., 61:7 (2018), 617–644  mathnet  crossref  crossref  adsnasa  isi  elib
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